Статья
2021
Dehydrogenation of Propane in the Presence of CO2 on Supported Monometallic MOy/SiO2 and CrOxMOy/SiO2 (M = Fe, Co, and Ni) Bimetallic Catalysts
M. A. Tedeeva, A. L. Kustov, P. V. Pribytkov, A. A. Strekalova, K. B. Kalmykov, S. F. Dunaev, L. M. Kustov
Российский журнал физической химии А
https://doi.org/10.1134/S0036024421010295
Abstract / Full Text
An analysis is performed of the physicochemical properties of M/SiO2 (M = Fe, Co, and Ni) oxide monometallic and CrM/SiO2 (M = Fe, Co, and Ni) bimetallic catalysts supported on amorphous silica. The catalysts are characterized via TGA, XRD, UV–Vis diffuse reflectance spectroscopy, and SEM. Adding 1 wt % of a second transition metal (Fe, Ni, and Co) to the 3% CrOx/SiO2 chromium oxide catalyst substantially raises the conversion of propane to 64% with a drop in the selectivity towards propylene and formation of methane as a main by-product in the case of nickel. Introducing iron and cobalt raises the selectivity towards propylene to 72% with a drop in the conversion of propane.
Author information
- Department of Chemistry, Moscow State University, 119991, Moscow, RussiaM. A. Tedeeva, A. L. Kustov, P. V. Pribytkov, K. B. Kalmykov, S. F. Dunaev & L. M. Kustov
- Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, 119334, Moscow, RussiaA. L. Kustov, P. V. Pribytkov & L. M. Kustov
- National University of Science and Technology (MISiS), 119049, Moscow, RussiaA. L. Kustov, A. A. Strekalova & L. M. Kustov
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